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2025-11-25 @ ALS 8.3.1

Overall Goals

  • Further optimize diffuse collection at 8.3.1
  • Lysozyme, Mac1 (P43 and C2), Huwe1 data collection
  • Mac1 soaks in both P43 and C2 spacegroups

Participants

  • In person: Kara, James, Mehagan
  • Remote: Justin and Joseph for processing, Steve for setting up OSN sync

Data

  • Root directory at ALS: /data/mcfuser/ucsf/fraser/25Nov2025/
  • Root directory on OSN: s3://diffuse-als-public/20251125/

Beamline Settings

Day 1 Parameters

Parameter Value Notes
X-ray energy 14000 eV @ 0.014 % bandwidth
Beam size 100 µm x 100 µm, circle pinhole.com 300
Defocused
Beam_defocused.jpg for profile
M1 moved from 2660 to 1980
M2 to compensate
Divergence - 0.6 x 0.1 mrad
Flux 1.73 x 10¹⁰ ph/s 860 Gy/s
But we are in decay mode of the ring so will drop over time
Beamstop standard 8.3.1
Data collection software Blu-Ice
Temperature control None, turned cryo stream off and moved out

Samples

Name Sample Well composition Drop composition Notes
Mac1 (P43) SARS CoV2 NSP3 macrodomain and seed stock. 40 mg/mL Mac1 in 150 mM NaCl, 20 mM Tris pH 8, 5% glycerol 34% (w/vol) PEG 3000 + 100 mM CHES (pH 9.5) 200 nL protein solution + 100 nL well solution + 100 nL seeds Galen setup
Reference PDB: 7TWF
Huwe1 (P43 21 2) 88 mg/mL NaCl 2-3.5M NaOac 50-200mM pH 4.84 200 nL protein solution + 200 nL well solution
Lysozyme 20 mg/mL From Hampton kit
30% PEG 5000, 1 M NaCl, 0.05 M Na Acetate trihydrate pH 4.6
Mac1 (C2) SARS CoV2 NSP3 macrodomain, 15 mg/mL Mac1 in 150 mM NaCl, 20 mM Tris pH 8, 5% glycerol 100 mM Tris pH 8.5, 100 mM Na Acetate, 28% PEG 4000 200 nL protein solution + 200 nL well solution Kara purified protein and setup 2 trays on 11/23
Reference PDB: 7KR0

Data collection, day 1

1. Lysozyme

Subdirectory: lysozyme/lysozyme_1

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
lysozyme_1 30 750 0.1 7200 0.01 175 Crystal slipped, aborted run

2. Mac1

Subdirectory: mac1/mac1_1

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_1 30 750 0.1 7200 0.01 175 Diffraction weaker than expected and some extra background rings, may need to clean beam path up here and possibly increase dose

Detector still paused around 7000 frames but eventually finished after writing out the data
mac1_1_bg 30 750 1 720 0.1 175 Went ~180 um away, rings still present - seems to be coming from collimator

Need to get rid of collimator rings - try lowering energy to see if that helps as a start

Note

Switching to 11.145 keV - will be higher dose rate

Parameter Value Notes
X-ray energy 11145 eV @ 0.014 % bandwidth
Beam size 100 µm x 100 µm, circle Divergence the same - 0.6 x 0.1 mrad
Some tune up after changing energy
Flux 3.26 x 10¹⁰ ph/s 2573 Gy/s
But we are in decay mode of the ring so will drop over time

3. Mac1

Subdirectory: mac1/mac1_2

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_2_data 0 720 0.1 7200 0.02 175 Increased exposure time to help the detector
Much better diffraction
Data got broken up into sweeps still
All data got written with no pause
mac1_2_bg 0 720 1 720 0.2 175 Moved 150 away

Based on XDS plots - for sure damaging beyond 440 deg (based on Garman limit), damaging more like 180 deg for R_d, might be okay

4. Mac1

Subdirectory: mac1/mac1_3

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_3_data 0 720 0.1 7200 0.02 175 Looking good
mac1_3_bg 0 720 1 720 0.2 175 Moved 150 away

5. Huwe1

Subdirectory: huwe1/huwe1_1

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
huwe1_1_data 0 720 0.1 7200 0.02 175 Looking good
huwe1_1_bg 0 720 1 720 0.2 175 Moved 250 away

Also looks like it survives to about 360

6. Huwe1

Subdirectory: huwe1/huwe1_2

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
huwe1_2_data 0 720 0.1 7200 0.02 175 Looking good
huwe1_2_data_2 0 720 0.1 7200 0.02 175 Moved 150 um away to take data on new spot on the crystal

Detector a little unhappy, paused in the middle a few times - will give multiple sweeps
huwe1_2_bg 0 720 1 720 0.2 175 Moved 300 away from second spot

James increased the ram limit to help

7. Huwe1

Subdirectory: huwe1/huwe1_3

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
huwe1_1_data 0 720 0.1 7200 0.02 175 Looking good and detector happier, wrote as one sweep
huwe1_1_bg 0 720 1 720 0.2 175 Moved 300 away

Mac1 - set up 3 soaks - 9 uL reservoir solution + 1 uL 200 mM ADPr (so final concentration is 20 mM) - First soak - starts at 0 min - Second soak - starts at 6 min - Third soak - starts at 11 min

8. Mac1

Subdirectory: mac1/mac1_4

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_4_data 0 720 0.1 7200 0.02 175
mac1_4_bg 0 720 1 720 0.2 175 Accidentally went into mac1_4_bg directory

Now at 1700 Gy/s, ring keeps decaying

9. Mac1

Subdirectory: mac1/mac1_5

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_5_data 0 720 0.1 7200 0.02 175
mac1_5_bg 0 720 1 720 0.2 175

Warning

Skip, crystal slipped

10. Mac1 + ADPr

Soaked with ADPr for ~50 min (9 uL + 1 uL)

Subdirectory: mac1/mac1_6

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_6_adpr_data 0 720 0.1 7200 0.02 175 All good
mac1_6_adpr_bg 0 720 1 720 0.2 175 All good, went 300 um away

Info

Quick check with XDS/dimple - looks like high ADPr occupancy

Shutters closed by ALS - finally refilling the ring

Beam back - tuneup.com
Flux - 5.922 x 10^10 ph/s, dose is 4668 Gy/s

11. Mac1 + ADPr

Soaked with for ~60 min (9 uL + 1 uL)

Subdirectory: mac1/mac1_7

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_7_adpr_data 0 720 0.1 7200 0.02 175 All good
mac1_7_adpr_bg 0 720 1 720 0.2 175 Went 250 um away

Quick check with XDS/dimple

fairly high occupancy, but not as high as Mac1_6

12. Lysozyme

Subdirectory: lysozyme/lysozyme_2

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
lysozyme_2_data 0 720 0.1 7200 0.02 175 All good
lysozyme_2_bg 0 720 1 720 0.2 175 Went 350 um away

13. Lysozyme

Subdirectory: lysozyme/lysozyme_3

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
lysozyme_3_data 0 720 0.1 7200 0.02 175 All good
lysozyme_3_bg 0 720 1 720 0.2 175 Went 200 um away

14. Mac1 + ADPr

Soaked with ADPr for ~15min (9 uL + 1 uL)

Subdirectory: mac1/mac1_8

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_8_adpr_data 0 720 0.1 7200 0.02 175 All good
mac1_8_adpr_bg 0 720 1 720 0.2 175 Went 200 um away

Quick check with XDS/dimple

density is there

15. Mac1 + ADPr

Soaked with ADPr for ~30min (9 uL + 1 uL)

Subdirectory: mac1/mac1_9

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_9_adpr_data 0 720 0.1 7200 0.02 175 All good
mac1_9_adpr_bg 0 720 1 720 0.2 175 Went 250 um away

Quick check with XDS/dimple

density is there

16. Mac1 + ADPr

Soaked with ADPr for ~20min (9 uL + 1 uL)

Subdirectory: mac1/mac1_10

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_10_adpr_data 0 720 0.1 7200 0.02 175 All good
mac1_10_adpr_bg 0 720 1 720 0.2 175 Went 200 um away

Quick check with XDS/dimple

pretty good occupancy - maybe due to smaller crystal?

17. Mac1 + ADPr

Soaked with ADPr for ~50min (9 uL + 1 uL)

Subdirectory: mac1/mac1_11

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_11_adpr_data 0 720 0.1 7200 0.02 175 All good
mac1_11_adpr_bg 0 720 1 720 0.2 175 Went 200 um away

Quick check with XDS/dimple

lower occupancy, maybe due to larger crystal?

Mac1 C2, 1 - test, skip

End of day 1

Data collection, day 2

11.26.2025

Starting with long Mac1 P43 soaks

  • AVI-3731 (opener) - 2 uL + 0.5 uL (100 mM stock) - some phase separation in the drop, probably due to DMSO? Let soak go 1-2 hrs - crystals cracked at ~1 hr mark, try again with shorter time or lower concentration
  • ADPr - 9 uL + 1 uL (200 mM stock) - let go 1-2 hrs

Dose rate: 4828 Gy/s

18. Mac1 + ADPr

Soaked with ADPr for ~90min (9 uL + 1 uL)

Subdirectory: mac1/mac1_12

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_12_adpr_data 0 720 0.1 7200 0.02 175 All good
mac1_12_adpr_bg 0 720 1 720 0.2 175 Went 200 um away - accidentally has 824 images because the data collection was incorrectly set for 7200 images and aborted

Quick check with XDS/dimple

ADPr density

Mac1, 13 - skip

19. Mac1 + AVI-3731

Added 100 nL directly to well H9 (multiple crystals) let sit for ~30 min

Subdirectory: mac1/mac1_14

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_14_avi3731_data 0 720 0.1 7200 0.02 175 All good
mac1_14_avi3731_bg 0 720 1 720 0.2 175 Went 200 um away

Quick check with XDS/dimple

Not sure what the compound is supposed to look like but there is positive density near V49, not many large sidechain motions though

20. Mac1 + AVI-3731

Added 100 nL directly to well H10 (multiple crystals) let sit for ~30 min

Subdirectory: mac1/mac1_15

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_15_avi3731_data 0 720 0.1 7200 0.02 175 All good
mac1_15_avi3731_bg 0 720 1 720 0.2 175 Went 200 um away

Quick check with XDS/dimple

for sure ligand density, not a ton of sidechain motions

At 60 min, crystals are dead for drops H9 and H10

For G10, added 200 nL of well solution and then 100 nL of AVI3731

Also made two drops - 4.5 uL each, transferred one crystal per drop, then added 0.5 uL of AVI3731 to the drop

21. Mac1 + AVI-3731

Added 200 nL reservoir + 100 nL AVI-3731 directly to well G10 (multiple crystals) let sit for ~45 min

Subdirectory: mac1/mac1_16

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_16_avi3731_data 0 720 0.1 7200 0.02 175 All good
mac1_16_avi3731_bg 0 720 1 720 0.2 175 Went 200 um away

Quick check with XDS/dimple

seeing large green density, not a lot of motions

22. Mac1 + AVI-3731

Made 4.5 uL drop of reservoir solution, added crystal, and then added 0.5 uL AVI-3731 (single crystal) let sit for ~45 min

Subdirectory: mac1/mac1_17

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_17_avi3731_data 0 720 0.1 7200 0.02 175 Diffraction a bit weaker than typical - looks like I only got a piece of the crystal
mac1_17_avi3731_bg 0 720 1 720 0.2 175 Went 400 um away

Quick check with XDS/dimple

larger green blob for ligand

23. Mac1 + AVI 3731

Made 4.5 uL drop of reservoir solution, added crystal, and then added 0.5 uL AVI-3731 (single crystal) let sit for ~60 min (second drop)

Subdirectory: mac1/mac1_18

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_18_avi3731_data 0 720 0.1 7200 0.02 175 Was able to loop the entire crystal, all good
mac1_18_avi3731_bg 0 720 1 720 0.2 175 Went 400 um away

Quick check with XDS/dimple

stronger ligand density and also some other peaks?

Made 2 more 4.5 uL drops, added crystal, and then added 0.5 uL of AVI 3731 - let sit for 1.5-2 hrs

Mac1 C2, 2 - lost it or not diffracting well, skip

24. Mac1 + AVI-3731

Made 4.5 uL drop of reservoir solution, added crystal, and then added 0.5 uL AVI-3731 (single crystal) let sit for ~120 min

Subdirectory: mac1/mac1_19

Prefix φ0 (deg.) φ1 (deg.) ∆φ (deg.) Images ∆t (s) d (mm) Notes
mac1_19_avi3731_data 0 720 0.1 7200 0.02 175 all good
mac1_19_avi3731_bg 0 720 1 720 0.2 175 Went 200 um away

Quick check with XDS/dimple

strong ligand density

done!

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